WISH I could remember my sources but - when I was in high school, I did a one of those Academy of Science projects on gasification - of *trash*. Basically, any trash that contained wood pulp or paper products. Stuff that'd burn. I started with destructive distillation to extract the alcohols, and then use the charcoal that was left to begin the rest of the process. I used to know the names of the processes - and all I can remember is it required super-heated steam and a few metallic catalysts along with the charcoal. It consumed some fuel to produce fuel, but being a high school student, I postulated that the source of the power could always have come from a nuclear reaction. So the steam was heated by nuclear power, and it made something CLOSE to gasoline.
My experiments produced only slightly flammable sludge, but the idea was good. We're NEVER gonna run out of trash. We could always just take someone ELSE's trash.
The supposition is one I've always maintained - octane - gasoline - really, really IS an outstanding fuel. It delivers a fantastic punch per liter, and it's very safe to transport. I didn't, and still don't think it'd be a waste of good, nuclear power to be converted into something transportable - and *storable*.
Anyway, it came in second place. That was almost thirty years ago.